西亚试剂：nanopatterns on metal-graphene hybrid materials

发布时间：2025-06-04

"We can generate nanopatterns on metal-graphene hybrid materials, which opens new ways to pattern 2-D crystals," Cheng said.

The technique works by using a pulsed laser to generate "high strain rate" imprinting of metals into the nanomold.

"We start with a metal thin film, and we can deform it into 3-D nanoshapes patterned over large areas," Cheng said. "What is more interesting is that the resulting 3-D nanostructures are still crystalline after the imprinting process, which provides good electromagnetic and optical properties."

Whereas other researchers have created nanoshapes out of relatively soft or amorphous materials, the new research shows how to create nanoshapes out of hard and crystalline metals.

The silicon nanomolds were fabricated at the Birck Nanotechnology Center in Purdue's Discovery Park by a research group led by Minghao Qi, an associate professor of electrical and computer engineering.

"It is counter-intuitive to use silicon for molds because it is a pretty brittle material compared to metals," Qi said. "However, after we deposit an ultrathin layer of aluminum oxide on the nanomolds, it performs extremely well for this purpose. The nanomolds could be reused many times without obvious damage. Part of the reason is that although the strain rate is very high, the shock pressure applied is only about 1-2 gigapascals."

The shapes were shown to have an "aspect ratio" as high as 5, meaning the height is five times greater than the width, an important feature for the performance of plasmonic metamaterials.

"It is a very challenging task from a fabrication point of view to create ultra-smooth, high-fidelity nanostructures," Qi says. "Normally when metals recrystallize they form grains and that makes them more or less rough. Previous trials to form metal nanostructures have had to resort to very high pressure imprinting of crystalline metals or imprinting amorphous metal, which either yeilds high roughness in crystalline metals or smooth surfaces in amorphous metals but very high electrical resistance. For potential applications in nanoelectronics, optoelectronics and plasmonics you want properties such as high precision, low electromagnetic loss, high electrical and thermal conductivity. You also want it to be very high fidelity in terms of the pattern, sharp corners, vertical sidewalls, and those are very difficult to obtain. Before Gary's breakthrough, I thought it unlikely to achieve all of the good qualities together."

 

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